Storing single photons in broadband vapor cell quantum memories

Single photons are an essential resource for realizing quantum technologies. Together with compatible quantum memories granting control over when a photon arrives, they form a foundational component both of quantum communication and quantum information processing. Quality solid-state single photon sources deliver on the high bandwidths and rates required for scalable quantum technology, but require memories that match these operational parameters. In this thesis, I report on quantum memories based on electromagnetically induced transparency and built in warm rubidium vapor, with such fast and high bandwidth interfaces in mind. I also present work on a heralded single photon source based on parametric downconversion in an optical cavity, operated in a bandwidth regime of a few 100s of megahertz. The systems are characterized on their own and together in a functional interface. As the photon generation process is spontaneous, the memory is implemented as a fully reactive device, capable of storing and retrieving photons in response to an asynchronous external trigger.
The combined system is used to demonstrate the storage and retrieval of single photons in and from the quantum memory. Using polarization selection rules in the Zeeman substructure of the atoms, the read-out noise of the memory is considerably reduced from what is common in ground-state storage schemes in warm vapor. Critically, the quantum signature in the photon number statistics of the retrieved photons is successfully maintained, proving that the emission from the memory is dominated by single photons. We observe a retrieved single-photon state accuracy of $g_{c,\,\text{ret}}^{(2)}=0.177(23)$ for short storage times, which remains $g_{c,\,\text{ret}}^{(2)}<0.5$ throughout the memory lifetime of $680(50)\,$ns. The end-to-end efficiency of the memory interfaced with the photon source is $\eta_{e2e}=1.1(2)\,\%$, which will be further improved in the future by optimizing the operating regime. With its operation bandwidth of $370\,$MHz, our system opens up new possibilities for single-photon synchronization and local quantum networking experiments at high repetition rates.