Recent Advances in Bioinspired Proton-Coupled Electron Transfer

Pannwitz, Andrea and Wenger, Oliver S.. (2019) Recent Advances in Bioinspired Proton-Coupled Electron Transfer. Dalton Transactions, 48 (18). pp. 5861-5868.

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Official URL: https://edoc.unibas.ch/73096/

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Mechanistic investigations of proton-coupled electron transfer (PCET) are increasingly important, especially in the context of small molecule activation and solar energy conversion. The main part of this invited Perspective discusses 16 mechanistic PCET studies published over the past 5 years that contributed significantly to understanding and controlling PCET in artificial systems. This includes bio-inspired work on tyrosine-Z mimics, reactions involving the transfer of multiple protons, de novo designed proteins with very long-lived tyrosyl radicals, and PCET in artificial DNA systems. Particular emphasis is on light-triggered reactions. An outlook into future directions for research on PCET is given at the end.
Faculties and Departments:05 Faculty of Science > Departement Chemie > Chemie > Anorganische Chemie (Wenger)
UniBasel Contributors:Wenger, Oliver and Pannwitz, Andrea
Item Type:Article, refereed
Article Subtype:Research Article
Publisher:Royal Society of Chemistry
Note:Publication type according to Uni Basel Research Database: Journal article
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Last Modified:10 Dec 2019 11:11
Deposited On:10 Dec 2019 11:11

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