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Stokes and anti-Stokes Raman spectra of the high-energy C-C stretching modes in graphene and diamond

Jorio, Ado and Kasperczyk, Mark and Clark, Nick and Neu, Elke and Maletinsky, Patrick and Vijayaraghavan, Aravind and Novotny, Lukas. (2015) Stokes and anti-Stokes Raman spectra of the high-energy C-C stretching modes in graphene and diamond. physica status solidi (b), 252 (11). pp. 2380-2384.

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Official URL: http://edoc.unibas.ch/39760/

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Abstract

The Stokes and the anti-Stokes Raman spectra from the high energy carbon–carbon stretching modes in graphene and diamond are studied, with a focus on their intensity dependence on the excitation laser power. For diamond, the experiment was performed on a 50 μm slice of chemical vapour deposition grown single crystal using a 785 nm laser, in both the continuous wave (CW) and pulsed mode-locked (ML—130 fs pulses) excitation regimes. For graphene, the experiments were performed on suspended samples, including single layer, bilayer with AB-staking, twisted bi-layer and a sample with 4–6 layers, using λ = 532 and 633 nm CW lasers. The Stokes and anti-Stokes intensities vary largely from sample to sample, and the anti-Stokes/Stokes intensity ratio shows different excitation laser power behaviours. These differences can be explained on the basis of laser heating or correlated Stokes–anti-Stokes scattering phenomena.
Faculties and Departments:05 Faculty of Science > Departement Physik > Physik > Georg H. Endress-Stiftungsprofessur für Experimentalphysik (Maletinsky)
UniBasel Contributors:Maletinsky, Patrick M.
Item Type:Article, refereed
Article Subtype:Research Article
Publisher:Wiley
ISSN:0370-1972
e-ISSN:1521-3951
Note:Publication type according to Uni Basel Research Database: Journal article
Language:English
Identification Number:
Last Modified:14 Dec 2017 07:46
Deposited On:28 Apr 2016 09:31

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